Synchronization of two passively mode-locked, picosecond lasers within 20 fs for coherent anti-Stokes Raman scattering microscopy

نویسندگان

  • David J. Jones
  • Eric O. Potma
  • Ji-xin Cheng
  • Yang Pang
  • Jun Yea
  • X. Sunney Xie
چکیده

We report on the synchronization of two commercial picosecond Ti:sapphire lasers with unprecedented low temporal jitter between the pulse trains. Pulse jitter is reduced from a few picoseconds to 20 fs with a stability of several hours. The technology enabling the tight pulse synchronization is reviewed in this article. We demonstrate the usefulness of the synchronization scheme by applying the technique to coherent anti-Stokes Raman scattering CARS microscopy. It is shown that CARS images can be acquired with a significant improvement in signal-to-noise ratio. This level of performance brings the fluctuations of the CARS signal down to the fundamental photon shot-noise limit. We present detailed statistical analysis of the pulse jitter and CARS noise along with enhanced CARS vibrational images of polymer beads. © 2002 American Institute of Physics. DOI: 10.1063/1.1492001

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

High-sensitivity coherent anti-Stokes Raman scattering microscopy with two tightly synchronized picosecond lasers.

We demonstrate a significant improvement in signal-to-noise ratio in coherent anti-Stokes Raman scattering (CARS) spectroscopy/microscopy, using two highly synchronized picosecond Ti:sapphire lasers. A temporal jitter between the pulse trains from the two independent commercial lasers is reduced from a few picoseconds to ~21 fs , maintained over several hours. The tight synchronization brings t...

متن کامل

Prolonged-excitation coherent Raman spectroscopy with spectral resolution beyond the transition linewidth using two tunable picosecond dye lasers

Received June 11, 1984; accepted September 20, 1984 A time-resolved coherent anti-Stokes Raman technique is demonstrated that yields a spectral resolution beyond the linewidth obtained in spontaneous Raman spectroscopy. Two picosecond dye lasers, independently tunable with low timing jitter, are used. The coherent material excitation is generated by long pump pulses and monitored by short delay...

متن کامل

Broadband coherent anti-Stokes Raman scattering spectroscopy of nitrogen using a picosecond modeless dye laser.

Broadband picosecond coherent anti-Stokes Raman scattering (CARS) spectroscopy of nitrogen is demonstrated using 145-ps pump and probe beams and a 115-ps Stokes beam with a spectral bandwidth of 5 nm. This is, to our knowledge, the first demonstration of broadband CARS using subnanosecond lasers. The short temporal envelope of the laser pulses and the broadband spectral nature of the Stokes bea...

متن کامل

LETTERS An Epi-Detected Coherent Anti-Stokes Raman Scattering (E-CARS) Microscope with High Spectral Resolution and High Sensitivity

Coherent anti-Stokes Raman scattering (CARS) microscopy provides a unique approach to imaging chemical and biological samples by using molecular vibrations as a contrast mechanism.1,2 CARS is a four-wave mixing process involving a pump beam and a Stokes beam, with center frequencies at ωp and ωs, respectively. When ωp ωs is tuned to be resonant with a given vibrational mode, an enhanced CARS si...

متن کامل

Communication: Time-domain measurement of high-pressure N2 and O2 self-broadened linewidths using hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering.

The direct measurement of self-broadened linewidths using the time decay of pure-rotational hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps RCARS) signals is demonstrated in gas-phase N(2) and O(2) from 1-20 atm. Using fs pump and Stokes pulses and a spectrally narrowed ps probe pulse, collisional dephasing rates with time constants as short as 2.5 ps are captured wit...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2002